Instead of those particular words perhaps I could say "self-sustainment" (i.e. biological systems, genetic programming) and the ability (not necessarily always used) to react to one's environment. Included in the second are things such as free will, instinct, etc. and provides the variability when referring to chaos.
Many cognitive scientists think that the yet unanswered questions about what consciousness, sentience, etc. are will be answered when neurons can be analyzed on the quantum level.
Perhaps chaos is that which cannot be defined (along with its "other side", order). What I can say is that I'm not using it as the opposite of what could be seen as the "clockwork of the universe". I don't think there is a clockwork in the universe, inexorably moving everything mechanically towards some end or another.
It doesn't have to be defined in order to be used as a concept. There are concepts such as that, e.g. "society". Society exists, but good luck defining it. Same thing with "species" (biological, not chemical).
Pointing out the quantum world, which can be seen as either perfectly ordered (albeit in a way which we cannot observe), or perfectly chaotic (but most definitely without a clockwork). I'm more of the mind that it is both... the superposition of chaos and order, perhaps just like life itself. Again, an analogy, if you will: on a quantum level, you can look (sort of) and see (well, not really, but you can assume) superpositions of certain binary states (why we assume they are binary is beyond me-- I'm more likely to believe they are infinite)... perhaps life, then, is a superposition of all states. What's meant by "all"? At each "point" in time (which I suppose doesn't exist at the limit), an infinite multiverse is 'created', and the superposition of all these states somehow gives life.
Everything is parenthetical to something else. So in the centre, you could 'see' the perfect order of quarks or whatever the heck is the particle of the hour (let's call it the of time Planck's constant instead hardy har har) [or is that perfect disorder?]... anway, moving outwards then you see molecules in perfect arrays of crystal stucture, but then each chunk being disordered, then the rock could be picked up and smashed.
lol - I've lost it.