@Airlane1979,
Yes, you are being unreasonable.
Quiet enjoyment of the premises also applies for your neighbor as well as you. You're not complaining of a loud tv volume, vacuuming or even fights that go on all night long.
The phone calls are during the day and interferes with no other building activity.
I suggest counseling to get a hold of these feelings that make you "insecure, invaded & frustrated." Somehow I don't think they're related to a neighbor talking on the phone to his family and friends.